Nucleic Acids in Chemistry and Biology

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produces the 2-monoalkylated nucleoside together with the 2,3-bis alkylated by-product. Subsequent
hydrolysis provides a simple and efficient route to 2-O-methylguanosine (Figure 3.38).^82
2 ,3-Dideoxynucleosideswere first prepared in the groups of Todd and Robins in the 1950s. More
recently, many such nucleoside derivatives have been discovered to have important anti-viral properties,
particularly effective against HIV (Section 3.4), and they have been used widely in DNA sequencing using
the Sanger method (Section 5.1). While glycosylation routes to these analogues are known, they generally
give anomeric mixtures of - and -nucleosides. A general route to these compounds via the correspond-
ing 2 ,3-didehydro-2,3-dideoxynucleosidesis shown in Figure 3.39.^83


Nucleosides and Nucleotides 99


PxO O

PxO

OHN

N

N
N

NHPx
HO O

HO NH 2

N

NH

N
N

O

NH 2
HO O

HO NHCOCF 3

N

NH

O

O

HO O

HO F

N

N

N
N

NH 2
HO O

HO NH 2

N

N

N
N

NH 2

(iii), (iv)
(i), (ii) (v), (iv)

Figure 3.35 Preparation of various 2-modified purine nucleosides. Reagents: (i) DAST, DMF, CH 3 CN (px pixyl/
9-phenylxanthyl); (ii) H; (iii) N^2 -palmitoyl guanine, bistrimethylsilyl acetamide, reflux; (iv) NH 3 /MeOH;
and (v) N^6 -octanoyl adenine, bistrimethylsilyl acetamide, reflux


4-MeOC 6 H 4 COO O N

N
O

O
Me
HO O

N 3

N

NH

O

O

Me

4-MeOC 6 H 4 COO O

HO

N

NH

O

O

Me

(i) (iii),(iv)

Figure 3.36 Synthesis of AZT via O^2 ,3-cyclonucleoside. Reagents: (i) i-PrO 2 CN^ NCO 2 i-Pr, Ph 3 P, DMF; (ii) LiN 3 ,
DMF; and (iii) NaOMe in MeOH


HO O

HO OMe

N

NH

O

O

HO O

HO OMe

N

N

NH 2

O

i-Pr

O

i-Pr
i-Pr

O

OH

N

NH

O

O

O

O

Si

Sii-Pr

N

N

O

O

NO 2

O

OMe

O

O

Si

Sii-Pr
i-Pr

O

i-Pr
i-Pr

(iii),(iv)

(i),(ii)
(v), (iv)

Figure 3.37 Syntheses of 2-OMe modified pyrimidine nucleosides. Reagents: (i) MeSO 2 Cl,DMAP then 2-nitrophenol;
(ii) MeI,Ag 2 O in acetone; (iii) 4-O 2 NC 6 H 4 CH^ NO.(Me 2 N) 2 C NH 2 then H 2 O/dioxan; (iv) TBAF in
THF; and (v) NH 3 in THF

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