Front Matter

(Tina Sui) #1
The two substrates (x-3 andx-6) with a pentadienyl system positioned at thex-6

position were oxygenated by SBLOX-1 at the highest rate, while the other three

substrates were oxygenated at 20 % (x-7), 25 % (x-5) and 60 % (x-4) of that of

AA (x-6).

The influence of the chain length of substrates bearing a 1Z,4Zpentadienyl system

located at thex-6 position was also studied in detail (Matsui et al., 1992) using an

entire series of (x 6 Z,x 9 Z)-C 13 C 24 dienoic acids and SBLOX-1 (Figure 6). It was

shown that the rates of oxygenation of the C 18 ,C 19 ,C 20 (maximum) and C 21 dienoic

acids were the highest. For C 17 and C 22 dienoic acids, the rates of oxygenation were

60 % of that of LA (C 18 ), while those of C 16 ,C 23 and C 24 dienoic acids fell between

20 % and 30 %. For lower chain lengths (C 15 ,C 14 and C 13 ) acids, the rates of oxy-

genation were insignificant.

Beside needing a correct positioning of the pentadienyl system around the n-6

position, SBLOX-1 substrates must also possess an anionic ionizable group at

one end of the carbon chain. While this requirement is fulfilled in natural substrates

by the presence of the carboxylate group, it has been shown that a sulfate group could

also be used (Bild et al., 1977a). By contrast, methyl esters (Hatanaka et al., 1984) or

triglycerides of PUFA are poor substrates for SBLOX-1, leading to low yields in

HPODs and a far less product specificity. Dienols synthesized by the reduction

of the carboxylate group of natural PUFAs are also oxygenated at a rate lower of

that of the parent compounds (20 % for example for the dienol arising from LA)

and with a far less product specificity (Hatanaka et al., 1989). On the other

hand, Brash and co-workers have shown that linoleic and arachidonic acids ester-

ified in phosphatidylcholine could be oxygenated by SBLOX-1 (20–30 % of the

rate of free acids) with no loss in product specificity (Brash et al., 1987). Finally, it

should be noted that anacardic acid (Figure 7), a constituent of cashew nut shells

(Anacardium occidentaleL.) is a substrate of SBLOX-1, with dioxygen being in-

serted at thex-4 position (Shoba et al., 1992).

16.3 Substrate and product specificities of lipoxygenases 345

Figure 6. Oxygenation of a series of (x 6 Z,x 9 Z)-C 13 C 24 dienoic acids catalyzed by SBLOX-1
(Matsui et al., 1992).


Figure 7. Anacardic acid, a substrate of SBLOX-1 (Shoba et al., 1992).

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