Wine Chemistry and Biochemistry

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6B Peptides 207


The amino acid composition of sparkling wine peptides depends on the aging


time (Moreno-Arribas et al. 1998b). The action of both types of proteases, but


mainly of the exocellular ones, that areactive in wines for months or even years,


causes large variations in peptide contents as happen during the aging of wines with


yeasts. Figures 6B.1 and 6B.2 illustrate these process showing the chromatograms


corresponding to the peptide fractions larger and smaller of 700 Da molecular mass,


respectively, of one must and the corresponding base wine and sparkling wines made


by thetraditionalmethod. It can be observed that, although the must hardly contains


any peptides in the fraction studied, their content increases during the production of


the base wine. The variation in the peptide content observed in the sparkling wines is


due to the successive and simultaneous degradation of some peptides and the release


of others during the aging with yeast.


Some of the lactic acid bacteria strains of wines have also shown proteolytic


activity in wine-making conditions (Feuillat et al. 1980; Manca de Nadra et al. 1997;


Leit ́ao et al. 2000). This activity has been found even in the presence of ethanol and


SO 2 (Manca de Nadra et al. 2005). It has been shown that this activity is greater in


red than in white wines (Manca de Nadra et al. 1999). The proteolytic activity is


a very important characteristic for some bacteria strains, allowing them to growth


in nitrogen-deficient media, and also favouring them to carry out malolactic fer-


mentation. According to Remize et al. (2005 and, 2006), peptides from 0.5 kDa to


10 kDa seem to be more favorable for the growth of wine lactic acid bacteria than


other nitrogen sources (<0.5 kDa). Alcaide-Hidalgo et al. (2008) have observed


a reduction in peptides during the malolactic fermentation of red wines followed
by an increase during the aging in barrels that was more evident when the aging


was in the presence of lees. The occurrence of proteolytic activity in all the stages


of wine manufacture can explain the wide range of peptides that can coexist in


a wine at any time and the discrepancies in most of the studies related to their


identification.


Glutathione is a peptide of non-proteic origin, present in grapes and wines that


merits a special mention. It was described for the first time in grapes by Cheynier


et al. (1989). Because of its strong antioxidant properties, it has been recommended


as an additive to prevent the enzymatic browning of white wines (Vaimakis and


Roussis 1996). Nevertheless, neither its evolution during wine manufacture nor its


precise role in wine manufacture are fully understood.


In an analysis of 29 varieties of grapes, Cheynier et al. (1989) detected glu-


tathione, mostly in a reduced form, GSH, at levels of 56.3–371.8μmol/kg in grapes


and of 41.9–332.7 mM in musts. According to Okuda and Yokotsuka (1999) and


Park et al. (2000), the glutathione content decreases during the firsts days of fer-


mentation, rising afterwards to reach values of 0.1–5.1 mg/L. According to Lavigne


et al. (2007), the amount of glutathione present in a wine at the end of the alcoholic


fermentation depends on the yeast strain, and decreases as the lees are removed and


also during the aging in barrels. In yeast, GSH accounts for about 1% of dry weight


ofSaccharomyces cerevisiaeand represents more than 95% of the low molecular


thiol pool (Elskens et al. 1991); thereby some of this glutathione could possibly be
released into the wine.

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