Wine Chemistry and Biochemistry

(Steven Felgate) #1

8D Yeasts and Wine Flavour 325


over use of SO 2 , stimulates glycerol production (Bataillon et al. 1996). Due to


its essential role as cofactor in the conversion of acetaldehyde to ethanol by alco-


hol dehy drogenase (Adhp), NADH oxidation depends on Gpdp activity, thereby


increasing glycerol formation (Radler and Sch ̈utz 1982). SO 2 addition to must


can also stimulate glycerol production by forming a hydroxysulfonate adduct with


acetaldehyde, again limiting NADH oxidation by Adhp, although the increase in


glycerol is relatively small at the rates of SO 2 addition in winemaking (Rankine and


Bridson 1971). Higher fermentation temperature, 25◦C compared to 15◦C, and


higher pH, 3.8 compared to 3.3, can increase glycerol production to a small extent


(Rankine and Bridson 1971).


8D.3.3 Non-volatile Organic Acids


8D.3.3.1 Significance


Acidity and pH constitute fundamental importance to the sensory perception of


wine, essentially defining its structure and balance. Excessive acidity increases the


perception of sourness whereas low acidity decreases flavour harmony. The percep-


tion of sourness and astringency of organic acids depends on concentration, pH and


anion species (Sowalsky and Noble 1998). Wine acidity is largely determined by
the major grape acidsL(+)-tartaric andL(–)-malic, with smaller contributions from


citric andD(–)-lactic acids. Grape acids can range from<5 g/L for over-ripened


grapes and exceed 10 g/L in early season grapes from cool regions intended for


sparkling wine, with 6–8 g/L usually being preferred for dry wines. Wine also


contains various non-volatileacids of microbial origin succinic, keto acids pyruvic


and -ketoglutaric,L(+)-lactic and lesser amounts of other non-volatile acids, which


contribute to acidity (Boulton et al. 1998; Fowles 1992). Volatile fatty acids of either


grape or microbial origin, which can further contribute to acidity and aroma, are


discussed in Sect. 8D.4.3


8D.3.3.2 Metabolism and Modulating Factors


Organic acid metabolism serves several important functions, as precursors for


biosynthetic pathways and in maintenance of redox balance. Of the major grape


acids, tartaric acid is not metabolised bySaccharomyces cerevisiaewhereasL-malic


acid can be partially degraded (3–45%) by most strains, but this pathway is restricted


by diffusion of the non-dissociated acid into the cell and active transport of malate


out of the cell (Salmon 1987). Several wine strains ofSaccharomyces cerevisiae


have a variable ability to produceL-malic acid, which can cause difficulties in pre-


dicting and controlling titratable acidity in new wines (Holgate 1997). Some strains


ofSaccharomyces bayanus/uvarumproduce malic acid, though this properties tends


to be strain dependent (Antonelli et al. 1999; Giudici et al. 1995).L-Malate is formed

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